Thermally Cross-Linkable Blended Hole Transport Layer for Solution-Processed Quantum Dot Light-Emitting Diodes
  • Kim, Dong Hyun
  • Lee, Kyung Jae
  • Hwang, Jeong Ha
  • Kwon, Haeju
  • Seo, Eunyong
  • ... Lim, Jaehoon
  • 외 5명
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초록

Solution-processed quantum-dot light-emitting diodes (QLEDs) are promising for next-generation display technology. However, the solution process challenges multilayer fabrication due to solvent-induced damage to underlying layers. We propose a robust and highly efficient hole transport layer (HTL) based on a cross-linked blend of N4,N4 '-Di(naphthalen-1-yl)-N4,N4 '-bis(4-vinylphenyl) biphenyl-4,4 '-Diamin (VNPB) and poly[bis(4-phenyl) (2,4,6-trimethylphenyl) amine] (PTAA). A precise control of the blend ratio allows a cross-linked structure with solvent resistance and tunable hole mobility and energy levels. The blended HTL, optimized at a 2:1 VNPB/PTAA ratio, outperforms nonblended VNPB or PTAA HTLs in QLEDs. This cross-linked blending strategy offers a promising approach for high-performance QLEDs by addressing electrical properties and solvent issues.

키워드

cross-linkinghole-transportlayerquantumdot light-emitting diode<italic>N</italic>4,<italic>N</italic>4 '-Di(naphthalen-1-yl)-<italic>N</italic>4,<italic>N</italic>4 '-bis(4-vinylphenyl) biphenyl-4,4 '-diamin (VNPB)poly[bis(4-phenyl) (2,4,6-trimethylphenyl) amine] (PTAA)STABILITY
제목
Thermally Cross-Linkable Blended Hole Transport Layer for Solution-Processed Quantum Dot Light-Emitting Diodes
저자
Kim, Dong HyunLee, Kyung JaeHwang, Jeong HaKwon, HaejuSeo, EunyongLee, JuwanMin, SinhuiCha, Ju-HongWhang, Dong RyeolLim, JaehoonLee, Donggu
DOI
10.1021/acsanm.5c02714
발행일
2025-08
유형
Article
저널명
ACS APPLIED NANO MATERIALS
8
34
페이지
16727 ~ 16735