Data-driven analysis in the selective oligomerization of long-chain linear alpha olefin on zeolite catalysts: A machine learning-based parameter study
  • "Lee, Sung Woo
  • Hidajat, Marcel Jonathan
  • Cha, Seung Hyeok
  • Yun, Gwang-Nam
  • Hwang, Dong Won
Citations

WEB OF SCIENCE

1
Citations

SCOPUS

1

초록

"In this study, the oligomerization of 1-octene was investigated using various zeolites through both experimental and machine learning (ML) approaches. The structural characteristics of the zeolites and experimental conditions were used as input parameters to analyze the feature importance of each key factor on the oligomerization of 1-octene. By quantifying these influences, the reaction mechanism was elucidated, and a methodology for maximizing the oligomerization reaction was developed. The ML methods employed in this study were SHapley Additive exPlanations (SHAP) and Sure Independence Screening and Sparsifying Operator (SISSO). While the SHAP method is a well-validated conventional approach, it has limitations due to its high data requirements. Therefore, the SISSO method was applied, as it requires fewer data points and offers a transparent computational process. SISSO provided results in the form of human-interpretable equations, allowing for an analysis of these equations to deepen insights into the reaction mechanism. © 2024 The Authors

키워드

IsomerizationMachine learningOligomerizationParameterSHAPSISSOHIGH-PERFORMANCE1-HEXENEIDENTIFICATIONPUBLICATIONS1-BUTENEZSM-5
제목
Data-driven analysis in the selective oligomerization of long-chain linear alpha olefin on zeolite catalysts: A machine learning-based parameter study
저자
"Lee, Sung WooHidajat, Marcel JonathanCha, Seung HyeokYun, Gwang-NamHwang, Dong Won
DOI
10.1016/j.fuproc.2024.108164
발행일
2025-03
유형
Article
저널명
Fuel Processing Technology
267