NaCl Microporogen-Assisted Hollow Microporous Organic Polymers Bearing Zn-Salphens for Enhanced Biomass Conversion to Biodiesel
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초록

Hollow microporous organic polymers bearing Zn-salphen species (HMOP-Zn) were engineered via template synthesis using micrometer-sized NaCl crystals as porogens. The NaCl porogens could be easily etched from NaCl@MOP-Zn by simple water washing without causing Zn etching from HMOP-Zn. HMOP-Zn was utilized as a heterogeneous Lewis acid catalyst for the transesterification of soybean oil with methanol to produce biodiesel. Due to the hollow morphology effect, HMOP-Zn exhibited superior catalytic performance compared to a control nonhollow MOP-Zn catalyst. In addition, HMOP-Zn could be recycled while maintaining its original catalytic activity for five successive reactions.

키워드

microporous organic polymerheterogeneous catalystzincsalphenbiomassbiodieselSOYBEAN OILTRANSESTERIFICATIONCATALYSTSPHERESOXIDE
제목
NaCl Microporogen-Assisted Hollow Microporous Organic Polymers Bearing Zn-Salphens for Enhanced Biomass Conversion to Biodiesel
저자
Lee, Jong DooKim, SeramSon, Seung Uk
DOI
10.1021/acsapm.5c01065
발행일
2025-05
유형
Article; Early Access
저널명
ACS APPLIED POLYMER MATERIALS
7
11
페이지
6635 ~ 6640