Two-Dimensional Metal-Insulator Transition in Ultrathin VO2 Nanosheets via Remote van der Waals Epitaxy
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초록

Vanadium dioxide (VO2) undergoes a rutile-to-monoclinic metal-insulator transition (MIT) at 340 K. Marked by abrupt resistivity changes of 10(4)-10(5) Omega<middle dot>cm, this property has long attracted interest for electronic applications. However, when VO2 is a few nanometers thick, substrate-induced strain destabilizes the MIT, which limits device performance. To overcome this, two-dimensional (2D) VO2 nanostructures grown with a remote distance from substrates can reveal intrinsic strain-free electrical behavior and enable high-performance MIT-based devices. We report the growth of few-nanometer-thick 2D VO2 via remote van der Waals epitaxy. Transmission electron microscopy confirmed the monoclinic (M1) crystal structure. Conductive atomic force microscopy (c-AFM) measurements demonstrated a complete onset of 2D MIT at 1.5 V, achieving an on/off ratio of nearly 10(4).

키워드

remote van der Waals epitaxyVO2nanosheetsmetal-insulator transitionvapor transfer methodOXIDES
제목
Two-Dimensional Metal-Insulator Transition in Ultrathin VO2 Nanosheets via Remote van der Waals Epitaxy
저자
Oh, Su-ArHeo, YuseongKim, Young-MinLim, Seong Chu
DOI
10.1021/acs.nanolett.5c05107
발행일
2026-02-04
유형
Article
저널명
Nano Letters
26
4
페이지
1261 ~ 1266